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documents/_static/css/custom.css

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+/* 
+Add brand colors here 
+
+See also: https://pydata-sphinx-theme.readthedocs.io/en/stable/user_guide/styling.html#color-variables
+*/
+html[data-theme="light"] {
+    --pst-color-primary: rgb(126, 3, 3);
+    --pst-color-secondary: rgb(218, 2, 2);
+}
+
+html[data-theme="dark"] {
+    --pst-color-primary: rgb(115, 199, 164);
+    --pst-color-secondary: rgb(21, 197, 124);
+}